In this paper we consider a complete connected noncompact Riemannian manifold
M with bounded geometry and spectral gap. We prove that the Hardy type spaces
X^k(M), introduced in a previous paper of the authors, have an atomic
characterization. As an application, we prove that the Riesz transforms of even
order 2k are bounded from X^k(M) to L^1(M)and on L^p(M) for 1<p<\infty.